Photoemission-time-delay measurements and calculations close to the 3s-ionization-cross-section minimum in Ar

Summary, in English

We present experimental measurements and theoretical calculations of photoionization time delays from the 3s and 3p shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using attosecond pulse trains and the infrared laser used for their generation. The theoretical approach includes intershell correlation effects between the 3s and 3p shells within the framework of the random-phase approximation with exchange. The connection between single-photon ionization and the two-color two-photon ionization process used in the measurement is established using the recently developed asymptotic approximation for the complex transition amplitudes of laser-assisted photoionization. We compare and discuss the theoretical and experimental results, especially in the region where strong intershell correlations in the 3s -> kp channel lead to an induced "Cooper" minimum in the 3s ionization cross section.

• Author: Diego Guenot; Kathrin Klünder; Cord Arnold; David Kroon; J. M. Dahlstrom; Miguel Miranda; Thomas Fordell; Mathieu Gisselbrecht; Per Johnsson; Johan Mauritsson; E. Lindroth; A. Maquet; R. Taieb; Anne L'Huillier; A. S. Kheifets
• Department/s: Atomic Physics; Synchrotron Radiation Research
• Publishing year: 2012
• Language: English
• Publication/Series: Physical Review A (Atomic, Molecular and Optical Physics)
• Volume: 85
• Issue: 5
• Full text: - 815 kB; Download statistics
• Links: http://dx.doi.org/10.1103/PhysRevA.85.053424
• Document type: Journal article
• Publisher: American Physical Society
• Topic: Atom and Molecular Physics and Optics
• Status: Published
• ISBN/ISSN/Other: ISSN: 1050-2947